Jeffrey, who hails from Goderich, began his NHL hockey career career in Detroit with the Red Wings in 1961. He also played with the New York Rangers and Toronto Maple Leafs.
It was with the Buds that Jeffrey won the Stanley Cup back in 1967.
Jeffrey retired from hockey in 1969.
Larry Jeffrey was 81.
No funeral arrangements have been announced as of yet.
Below is a short profile on Jeffrey from the The Staysh.